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Bulky cyclopentadienyl ligands

In the area of organometallic chemistry, a bulky cyclopentadienyl ligand is jargon for a ligand of the type C5H5−nR−n where R is a branched alkyl and n = 3 or 4. Representative examples are the tetraisopropyl derivative C5HiPr−4 and the tris(tert-butyl) derivative 1,2,4-C5H2tBu−3. These ligands are so large that their complexes behave differently from the analogues derived from pentamethylcyclopentadienyl, itself a bulky ligand.

General properties of complexes
Because they cannot closely approach the metal, these bulky ligands can stabilize high spin complexes, such as (C5H2tBu3)2Fe2I2. These large ligands stabilize highly unsaturated derivatives such as (C5H2tBu3)2Fe2N2. ==Synthesis and reactions==
Synthesis and reactions
. This compound is conveniently prepared by alkylation of cyclobutadiene with tert-butyl bromide under phase-transfer conditions. In contrast to (C5Me5)2Ir2Cl4, (tBu3C5H2)IrCl2 is monomeric. ==Related bulky ligands==
Related bulky ligands
Less bulky ligand are of the type where R is a branched alkyl. Examples include the di-tert-butyl and related trimethylsilyl derivatives. One such complex is . ==References==
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