In 2005, Smith, together with her sister Leah, decided to record their first album,
Leah and Chloe, one afternoon in the basement studio of a friend. The album was meant as a gift for family and friends but they received so much support and recognition for it that they decided to officially start a band called Rising Appalachia. Smith said of the experience: In the early days, the sisters
busked in the
French Quarter of New Orleans and elsewhere. They began to find their own natural interpretation of
Appalachian music which brought together folk, soul,
hip-hop,
classical,
southern gospel and other styles based on their upbringing on traditional Appalachian
string band music, as well as on their exposure to urban music like hip-hop and
jazz and the influence of
roots music of all kinds which they experienced during their worldwide travels. The sisters integrate live performance art into
Rising Appalachia's shows. Speaking about this, Smith said: ==Natural medicine and healing==