MarketCrystal twinning
Company Profile

Crystal twinning

Crystal twinning occurs when two or more adjacent crystals of the same mineral are oriented so that they share some of the same crystal lattice points in a symmetrical manner. The result is an intergrowth of two separate crystals that are tightly bonded to each other. The surface along which the lattice points are shared in twinned crystals is called a composition surface or twin plane.

Definition
Twinning, a version of macle, is a form of symmetrical intergrowth between two or more adjacent crystals of the same mineral. It differs from the ordinary random intergrowth of mineral grains in a mineral deposit, because the relative orientations of the two crystal segments show a fixed relationship that is characteristic of the mineral structure. The relationship is defined by a symmetry operation called a twin operation. The twin operation is not one of the normal symmetry operations of the untwinned crystal structure. For example, the twin operation may be reflection across a plane that is not a symmetry plane of the single crystal. On the microscopic level, the twin boundary is characterized by a set of atomic positions in the crystal lattice that are shared between the two orientations. These shared lattice points give the junction between the crystal segments much greater strength than that between randomly oriented grains, so that the twinned crystals do not easily break apart. Parallel growth describes a form of crystal growth that produces the appearance of a cluster of aligned crystals which could be mistaken for twins. Close examination reveals that the cluster is actually a single crystal. This is not twinning, since the crystal lattice is continuous throughout the cluster. Parallel growth likely takes place because it reduces system energy. ==Twin laws==
Twin laws
Twin laws are symmetry operations that define the orientation between twin crystal segments. These are as characteristic of the mineral as are its crystal face angles. For example, crystals of staurolite show twinning at angles of almost precisely 90 degrees or 30 degrees. It is possible for a rotational twin law to share the same axis as a rotational symmetry of the individual crystal if the twin law is a 2-fold rotation and the symmetry operation is a 3-fold rotation. This is the case for spinel law twinning on : The spinel structure has a 3-fold rotational symmetry on and spinel is commonly twinned by 2-fold rotation on . In the isometric system, the most common types of twins are the Spinel Law (twin plane, parallel to an octahedron) , where the twin axis is perpendicular to an octahedral face, and the Iron Cross , which is the interpenetration of two pyritohedrons, a subtype of dodecahedron. In the hexagonal system, calcite shows the contact twin laws {0001} and {0112}. Quartz shows the Brazil Law {1120}, and Dauphiné Law , which are penetration twins caused by transformation, and Japan Law {1122}, which is often caused by accidents during growth. In the tetragonal system, cyclical contact twins are the most commonly observed type of twin, such as in rutile titanium dioxide and cassiterite tin oxide. In the orthorhombic system, crystals usually twin on planes parallel to the prism face, where the most common is a {110} twin, which produces cyclical twins, such as in aragonite, chrysoberyl, and cerussite. In the monoclinic system, twins occur most often on the planes {100} and {001} by the Manebach Law {001}, Carlsbad Law [001], Baveno Law {021} in orthoclase, and the Swallow Tail Twins (Manebach law) {001} in gypsum. In the triclinic system, the most commonly twinned crystals are the feldspar minerals plagioclase and microcline. These minerals show the Albite and Pericline Laws. The most common twin operations by crystal system are tabulated below. This list is not exhaustive, particularly for the crystal systems of lowest symmetry, such as the triclinic system. ==Types of twinning==
Types of twinning
Simple twinned crystals may be contact twins or penetration twins. Contact twins meet on a single composition plane, often appearing as mirror images across the boundary. Plagioclase, quartz, gypsum, and spinel often exhibit contact twinning. An example is metazeunerite. Contact twinning characteristically creates reentrant faces where faces of the crystal segments meet on the contact plane at an angle greater than 180°. Rutile, aragonite, cerussite, and chrysoberyl often exhibit cyclic twinning, typically in a radiating pattern. :#parallel twinning, when the twin axis and compositional plane lie parallel to each other, :#normal twinning, when the twin plane and compositional plane lie normally, and :#complex twinning, a combination of parallel twinning and normal twinning on one compositional plane. ==Modes of formation==
Modes of formation
There are three modes of formation of twinned crystals. • Growth twins are the result of an interruption or change in the lattice during formation or growth. This may be due to a larger substituting ion, statistics as the energy difference to nucleate a new plane of atoms in a twin orientation is small, or because the twins lead to a lower energy structure. • Annealing or transformation twins are the result of a change in crystal system during cooling as one form becomes unstable and the crystal structure must re-organize or transform into another more stable form. • Deformation or gliding twins are the result of stress on the crystal after the crystal has formed. Because growth twins are formed during the initial growth of the crystal, they are described as primary, whereas transformation or deformation twins are formed in an existing crystal and are described as secondary. Growth twinning (nanotwinning) in a gold nanoparticle (electron microscope micrograph). There are two types of twinning that can occur during growth, accidental and ones where the twinned structure has lower energy. In accidental growth twinning an atom joins a crystal face in a less than ideal position, forming a seed for growth of a twin. The original crystal and its twin then grow together and closely resemble each other. This is characteristic enough of certain minerals to suggest that it is thermodynamically or kinetically favored under conditions of rapid growth. These cyclic twins occur as they are lower in energy at small sizes. For the five-fold case shown, there is a disclination along the common axis which leads to an additional strain energy. Balancing this there is a reduction in the surface free energy, in large part due to more (111) surface facets. In small nanoparticles the decahedral and a more complicated Icosahedral structure (with twenty units) are lower energy, but at larger energies single crystals become lower energy. However, they do not have to transform into single crystals and can grow very large, and are known as fivelings, documented as early as 1831 by Gustav Rose; further drawings are available in the Atlas der Kristallformen, and see also the article on fivelings. Transformation twinning Transformation and annealing twinning takes place when a cooling crystal experiences a displacive polymorphic transition. For example, leucite has an isometric crystal structure above about , but becomes tetragonal below this temperature. Any one of the three original axes of a crystal can become the long axis when this phase change takes place. Twinning results when different parts of the crystal break their isometric symmetry along a different choice of axis. This is typically polysynthetic twinning, which enables the crystal to maintain its isometric shape by averaging out the displacement in each direction. This produces a pseudomorphic crystal that appears to have isometric symmetry. Potassium feldspar likewise experiences polysynthetic twinning as it transforms from a monoclinic structure (orthoclase) to a triclinic structure (microcline) on slow cooling. In fcc metals, slip is almost always dominant because the stress required is far less than twinning stress. Twinning can occur by cooperative displacement of atoms along the face of the twin boundary. This displacement of a large quantity of atoms simultaneously requires significant energy to perform. Therefore, the theoretical stress required to form a twin is quite high. It is believed that twinning is associated with dislocation motion on a coordinated scale, in contrast to slip, which is caused by independent glide at several locations in the crystal. Compared to slip, twinning produces a deformation pattern that is more heterogeneous in nature. This deformation produces a local gradient across the material and near intersections between twins and grain boundaries. The deformation gradient can lead to fracture along the boundaries, particularly in bcc transition metals at low temperatures. Of the three common crystalline structures bcc, fcc, and hcp, the hcp structure is the most likely to form deformation twins when strained, because they rarely have a sufficient number of slip systems for an arbitrary shape change. High strain rates, low stacking-fault energy and low temperatures facilitate deformation twinning. If a metal with face-centered cubic (fcc) structure, like Al, Cu, Ag, Au, etc., is subjected to stress, it will experience twinning. The formation and migration of twin boundaries is partly responsible for ductility and malleability of fcc metals. Twin boundaries are partly responsible for shock hardening and for many of the changes that occur in cold work of metals with limited slip systems or at very low temperatures. They also occur due to martensitic transformations: the motion of twin boundaries is responsible for the pseudoelastic and shape-memory behavior of nitinol, and their presence is partly responsible for the hardness due to quenching of steel. In certain types of high strength steels, very fine deformation twins act as primary obstacles against dislocation motion. These steels are referred to as 'TWIP' steels, where TWIP stands for twinning-induced plasticity. Deformation twinning crystallography Twinning is crystallographically defined by its twin plane 𝑲𝟏, the mirror plane in the twin and parent material, and 𝜼𝟏, which is the twinning shear direction. During twinning, in addition to the twin plane, one more crystallographic plane ( 𝑲2) and a direction (𝜼2) onto that plane remain undistorted but rotated. Deformation twins in Zr are generally lenticular in shape, lengthening in the 𝜼𝟏 direction and thickening along the 𝑲𝟏 plane normal. The twin plane, shear direction, and shear plane form the basis vectors of an orthogonal set. The axis-angle misorientation relationship between the parent and twin is a rotation of angle 𝜉 about the shear plane's normal direction 𝑷. More generally, twinning can be described as a 180° rotation about an axis (𝑲𝟏 for type I twins or 𝜼𝟏 for type II twins normal direction), or a mirror reflection in a plane (𝑲𝟏 or 𝜼𝟏 normal plane). In addition to a homogeneous shear, atomic shuffles are sometimes required to reform the correct crystal structure in the twinned lattice. For each twin variant, a reciprocal twin with swapped 𝑲𝟏 and 𝑲2, 𝜼𝟏 and 𝜼2 is possible, but one variant may appear more frequently in reality due to complexities with the required shuffles. there are only two crystallographic planes in a shearing action that do not change their shape and size as a consequence of the shear. The first 𝑲𝟏 is the plane defining the upper and lower surfaces of the sheared volume. This plane contains the shear direction. The other plane, designated C. The shear direction is shown with an arrow and labelled with its customary designation 𝜼𝟏. It follows from the above that there are three ways that a crystal lattice can be sheared while still retaining its crystal structure and symmetry: • When 𝑲𝟏 is a rational plane and 𝜼2 a rational direction, a twin of the first kind • When 𝑲2 is a rational plane and 𝜼𝟏 a rational direction, a twin of the second kind, rare • When all four elements 𝑲𝟏, 𝑲2, 𝜼𝟏, and 𝜼2 are rational, a compound twin Deformation twinning configuration A deformation twin embryo forms in BCC metal by accumulating stacking faults, with a variant selection governed by the local stress state. Variation of the stress field close to twins inferred from HR-EBSD experimental and crystal plasticity finite element (CPFE) simulation data indicated that twins nucleate on sites with maximum strain energy density and twin resolved shear stress; thus, reducing the total elastic energy after formation. This relaxation depends on the twin thickness and is a deciding factor in the spacing between twins. Experimental and three-dimensional analysis has focussed on the (stored) strain energy density measured along a path. This highly localised stress field can provide a sufficient driving force for concurrent twin nucleation and inter/intra-granular crack nucleation. Deformation twin growth can be perceived as a two-step process of i) thickening that is mediated by the interaction between the residual and mobile twin partials at the coherent twin-parent interface, and ii) dislocation mobility along the twin shear direction. The twin propagates when the homogeneous shear stress reaches a critical value, and a twin-parent interface advances inside the parent grain [240]. The propagating deformation twin generates a stress field due to its confinement by the surrounding parent crystal, and deformation twins develop a 3D oblate spheroid shape (which appears in 2D sections as a bi-convex lens) with a mixed coherent and non-coherent interface (Figure b). found, using in-situ ultra-high-speed optical imaging, that twin nucleation in single-crystal magnesium is stress-driven accompanied by instantaneous propagation at a speed of 1 km/s (initially) that prioritises volume lateral thickening over forward propagation, past a critical width where growth is then become faster along the shear direction. Barnett also indicated that growth is due to twin tip extension. Furthermore, elastic simulations of the local stress field surrounding the ellipsoidal twin tip find that the field can be described using its lens angle (\beta) and that the stress field magnitude increases with twin thickness. diode (FSD) image for deformation twins at grain boundary in age-hardened ferrite at I) 18 mm working distance and II) 38 mm working distance. (b) Schematic of a lenticular twin with interface dislocations and (c) Twin band.|376x376px In practice, plastic accommodation occurs in the parent crystal; thus, it also depends on the material's yield stress, the anisotropic elastic stiffness of the parent crystal lattice, and the deformation twinning shear magnitude. A linear variation has been observed between twin thickness, stacking fault energy and grain size, and to a lesser degree, the stress state of the twinning grain (Schmid Factor). The twin thickness saturated once a critical residual dislocations' density reached the coherent twin-parent crystal boundary. Significant attention has been paid to the crystallography, morphology and macro mechanical effects of deformation twinning. Although the criterion for deformation twin growth is not entirely understood, it is a tip-controlled phenomenon linked to the interaction between the residual and mobile twin partials at the twin interface; thermodynamically, this involves the elastic energy of the strained lattice, the interface and volume free-energy of the twin, and the dissipated energy of the growth mechanism. To fully understand the interactions between microstructure (i.e., grain size, texture), temperature and strain rate on deformation twinning, it is crucial to characterise the (high) local stress and strain field associated with twin thickening and propagation. This is especially important for materials where cleavage fracture can be initiated by twinning (e.g., iron-silicon, the ferrite phase of age-hardened duplex stainless-steel, and single-crystal magnesium) as a stress-relieving mechanism. Early studies of deformation twins arrested within grains of niobium and iron visualised the highly local strain concentration at the twin tip using an etch-pit procedure. More recently, high-resolution electron backscatter diffraction (HR-EBSD) has been used to investigate the strain 'singularity' ahead of a twin tip in hexagonal close-packed (HCP) zirconium alloy. A deformation twin in commercial purity titanium was characterised similarly and then quantified using a local Schmid factor (LSF) at the twin tip, as described in equation below. \mathrm{LSF} = \frac{\boldsymbol{\sigma} : \boldsymbol{P}^i}{\|\boldsymbol{\sigma}\|}, \quad \boldsymbol{S}^i = \boldsymbol{d}^i \otimes \mathbf{n}^i where σ is the stress tensor, Si is the Schmid tensor, Pi is its symmetric part, di is the shear direction and ni is the shear plane normal for ith slip system. The authors concluded that conditions at the twin tip control thickening and propagation in a manner analogous to the operation of dislocation sources ahead of a crack-tip. In the analysis, a broad region of high LSF ahead of the twin tip favoured propagation, whereas a narrow region of high LSF promoted thickening. Since then, it has been argued that the LSF firmly controls the twin variant selection, as twinning has strong polarity. The LSF novelty – compared to other criteria to describe conditions at the twin so a suitable analysis method is needed. Lloyd who considered microscopic phase-field (MPF) models of cracks, noted that the stress fields were similar for dislocations, deformation twinning and martensitic transformations, with differences only in the traction of the created surface, i.e., there is 100% traction recovery for dislocations and a traction-free surface for a crack. They highlighted that the stress field singularity regulates the advancement of the crack-tip and dislocations. This stress concentration can be characterised using a path-independent line integral, as shown by Eshelby for dislocations considering the contribution from the surface traction and ellipsoidal inclusions, and Rice for cracks and stress concentrations with traction-free surfaces. Furthermore, Venables noted that the oblate spheroid shape of the twin tip is the ideal example of an ellipsoid inclusion or a notch. == See also ==
tickerdossier.comtickerdossier.substack.com