He then moved to the
University of Maryland, where he became chair of the Department of Physics and Astronomy in 1953. During his tenure as chair, he was responsible for a major increase in size and quality of the department. The physics building at the University of Maryland is named for him. In 1965 he left to become the second president of the
State University of New York at Stony Brook, a position he held until 1978. While he was there, Stony Brook University, one of four
SUNY centers created by then-governor
Nelson Rockefeller (briefly Vice President of the United States under
Gerald Ford), and, until recently, the only four allowed to call themselves "universities", grew to more than 17,000 students from a handful who started their academic careers before the campus was even finished, at the now-defunct State University of New York on Long Island (SUCOLI). He then returned to the University of Maryland to become president of the original five campuses of the University of Maryland. Comparable to a chancellor position in other
state university systems, at the time Toll oversaw the
University of Maryland, College Park,
University of Maryland, Baltimore County,
University of Maryland University College,
University of Maryland, Eastern Shore, and
University of Maryland at Baltimore. When
Governor William Donald Schaefer decided to merge most of the state's public universities into a single system, Toll was put in charge of the merger. He then became the first chancellor of the new
University System of Maryland. In 1995, at age 71, he became president of
Washington College, a small, private
liberal arts school in
Chestertown, Maryland. There, he was credited with fixing the school's budget crisis and raising its national profile. As a physicist, Toll was known for his work in
dispersion theory and
elementary particle physics. Between university jobs in the early 1990s, he was president of the
Universities Research Association which oversaw the U.S.
Superconducting Supercollider project until
Congress defunded it. In January 2004, he announced that he would leave Washington College and return to physics research at the University of Maryland. ==Personal life==