Villafurte was an assemblyman in the
Batasang Pambansa from 1978 to 1986. He also served as the
Minister of Trade in the cabinet of President
Ferdinand Marcos from 1979 to 1981. However, he then broke with Marcos and joined the opposition
UNIDO party. While campaigning for him during the
1984 Philippine parliamentary election, his sister-in-law Rosita Villafuerte, who was also the Vice Mayor of
Sipocot, Camarines Sur, was assassinated after speaking at a rally. After Marcos was overthrown in 1986, Villafuerte served as Secretary of Government Reorganization under President
Corazon Aquino. He defeated singer and actress
Nora Aunor to win his third and final term as governor, ending in 2004. At the same time, Villafuerte was the first president of the
League of Provinces of the Philippines from 1988 to 1990 and from 1998 to 2004. During his tenure, Villafuerte was accused of involvement in the
Fertilizer Fund scam, but was acquitted in 2018. In 2004, he was elected to the House of Representatives representing Camarines Sur and served until 2013. He also supported proposals to split parts of Camarines Sur into a separate province to be called Nueva Camarines, which resulted in a feud with his son and successor as governor,
Luis Raymund Villafuerte. In 2013, he ran again for governor but lost to his grandson
Miguel Luis Villafuerte, which occurred during a falling-out between the two in which the latter was supported by his father, Luis Raymund. The three reconciled in 2018. ==Personal life and death==