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Phosphorus sulfides

Phosphorus sulfides comprise a family of inorganic compounds containing only phosphorus and sulfur. These compounds have the formula P4Sn with n ≤ 10. Two are of commercial significance, phosphorus pentasulfide, which is made on a kiloton scale for the production of other organosulfur compounds, and phosphorus sesquisulfide, used in the production of "strike anywhere matches".

Preparation
The main method for preparing these compounds is thermolysis of mixtures of phosphorus and sulfur. The product distributions can be analyzed by 31P-NMR spectroscopy. More selective syntheses entail: • desulfurization, e.g. using triphenylphosphine and, complementarily, • sulfidation using triphenylarsine sulfide. ====== Phosphorus sesquisulfide is prepared by treating red phosphorus with sulfur above 450 K, followed by careful recrystallization with carbon disulfide and benzene. An alternative method involves the controlled fusion of white phosphorus with sulfur in an inert, non-flammable solvent. ====== The α- and β- forms of can be prepared by treating the corresponding isomers of with : The respective product distribution is then analyzed by using 31P-NMR spectroscopy. In particular, α- can be easily made by the photochemical reaction of with red phosphorus. ====== can be made by abstracting a sulfur atom from using triphenylphosphine: ====== is most conveniently made by direct union of the corresponding elements, and is one of the most easily purified binary phosphorus sulfides. : ====== β- can be made by treating α- with in , which yields a mixture between α- and β-. : ==See also==
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