In 1938, Boys was appointed an Assistant Lecturer in
Mathematical Physics at
Queen's University Belfast. He spent the whole of the
Second World War working on explosives research with the
Ministry of Supply at the
Royal Arsenal,
Woolwich, with Lennard-Jones as his supervisor. After the war, Boys accepted an
ICI Fellowship at Imperial College, London. In 1949, he was appointed to a Lectureship in
theoretical chemistry at the University of Cambridge. He remained at Cambridge until his death. He was only elected to a Cambridge College Fellowship at University College, now
Wolfson College, Cambridge, shortly before his death. Boys is best known for the introduction of
Gaussian orbitals into
ab initio quantum chemistry. Frank Boys was also one of the first scientists to use digital computers for calculations on polyatomic molecules. An International Conference, entitled "Molecular Quantum Mechanics: Methods and Applications" was held in memory of S. Francis Boys and in honour of
Isaiah Shavitt in September 1995 at
St Catharine's College, Cambridge. ==Awards and honours==