In the mid-1890s Tall Chief played an integral role in the introduction of the Peyote Religion or Native American Church to the Quapaw and Osage people. The Big Moon variant of the Native American Church was founded by a Caddo and Delaware man known as
John Wilson, who was also referred to as Moonhead. Wilson had been instructing the
Delaware People in this ceremony when Tall Chief heard of it. Tall Chief requested Wilson to show him this ceremony, which resulted in Wilson officiating a peyote ceremony for Tall Chief near present-day Skiatook, OK. Tall Chief invited several Osage Chiefs, who then went on to embrace this religion. Tall Chief also had Wilson introduce the ceremony to the group of Quapaw people who were living near the Spring River in what is now
Quapaw, OK. Tallchief was instructed by Wilson and became a Roadman. Tallchief had a roundhouse where he held Native American Church meetings near Skiatook, OK, and in Quapaw, OK on his allotment, and also put down Native American Church fireplaces for several families among the Osage and Quapaw people. ==Death and legacy==