Moore was born in Ireland and trained for a career as a civil engineer. He left for South Australia in 1861 When Moore took the position, the school had 12 pupils, the number growing during his incumbency to around 300. He retired in 1883, and on 22 February 1883 was honoured at a presentation ceremony.
Religious Moore took holy orders in 1880 While headmaster of Pulteney Street School, he also served as curate of
St Bartholomew's Church, Norwood, 1880–1881 and
St John's Church, Adelaide 1881–1884. From 1884 to 1900 he was rector of
St Mary's,
South Road, coupled with oversight of Christ Church, O'Halloran Hill, following the resignation of Rev.
C. H. Young. Over that period he was similarly attached to St George's Church, Goodwood. ==Death and recognition==